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In the simplest interacting boson model (IBM-1) [1], valence nucleon-pair coupling to angular momentum
$ L=0 $ and$ L=2 $ are mapped to s and d bosons. Many features of even-even nuclei can be elegantly described with up to two-body interactions. With a consistent-Q formalism often used in this model [2–4],$ \hat{H}_{1}=c\left[(1-\eta) \hat{n}_{d}-\frac{\eta}{N}\hat{Q}_{\chi}\cdot \hat{Q}_{\chi}\right], $
(1) it can produce the spectra of spherical (
$ \eta=0 $ ,$ U(5) $ limit), prolate ($ \eta=1 $ ,$ \chi=-{\sqrt{7}}/{2} $ ,$S U(3)$ limit), oblate ($ \eta=1 $ ,$ \chi={\sqrt{7}}/{2} $ ,$\overline{S U(3)}$ limit), and γ-soft ($ \eta=1 $ ,$ \chi=0 $ ,$ O(6) $ limit) nuclei. Here,$ \hat{n}_{d} $ is the d-boson number operator,$ \hat{Q}_{ \chi}=[d^{\dagger}\times\tilde{s}+s^{\dagger}\times \tilde{d}]^{(2)}+\chi[d^{\dagger}\times \tilde{d}]^{(2)} $ is the generalized quadrupole operator, N is the total boson number, c is a fitting parameter, and$ 0\leq \eta \leq 1, -{\sqrt{7}}/{2}\leq \chi \leq {\sqrt{7}}/{2} $ . This Hamiltonian can be also exploited to describe the shape transitional behaviors between these typical collective excitation modes. An interesting result is that, when$ \eta=1 $ and χ changes from$ -{\sqrt{7}}/{2} $ to${\sqrt{7}}/{2} $ , γ-soft rotation can be observed as a critical property between the prolate and oblate shapes [5] (Fig. 1). This means that triaxiality may result from the competition between the prolate and oblate shapes.Figure 1. (color online) Partial phase diagram in the cubic-Q interacting boson model Hamiltonian
$ \hat{H}_{2} $ .However, this simple Hamiltonian cannot describe γ-rigid triaxial deformation. This deficiency can be overcome by considering higher-order interactions [6, 7].
$ [d^{\dagger}d^{\dagger}d^{\dagger}]^{(L)}\cdot[\tilde{d}\tilde{d}\tilde{d}]^{(L)} $ interactions have been investigated and can result in a stable γ-rigid triaxial deformation for the ground state of a nucleus. Subsequently,$S U(3)$ symmetry-conserving higher-order interactions have also been systematically investigated [8], and a realization of the rigid quantum asymmetric rotor within the$S U(3)$ limit was established [9, 10]. These studies discussed the functions of the$S U(3)$ third-order interactions ($ [\hat{Q}\times \hat{Q}\times \hat{Q}]^{(0)} $ ,$ [\hat{L}\times \hat{Q}\times \hat{L}]^{(0)} $ ) and fourth-order interactions ($ (\hat{Q}\cdot \hat{Q})^{2} $ ,$ [(\hat{L}\times \hat{Q})^{(1)}\times (\hat{L}\times \hat{Q})^{(1)}]^{(0)} $ ), where$ \hat{Q}=\hat{Q}_{-{\sqrt{7}}/{2}} $ is the$S U(3)$ quadrupole operator.$S U(3)$ third-order and fourth-order interactions are also discussed in Refs. [11–15]. These interactions can remove the degeneracy in the γ-band and β-band of the spectra within the$S U(3)$ limit and are also intimately connected with the rigid triaxial rotational spectra. Higher-order terms are also important in partial dynamical symmetry [16]. Isacker demonstrated that higher-order interactions$ (\hat{Q}_{0}\times\hat{Q}_{0}\times\hat{Q}_{0})^{(0)} $ can be individually used to present a rotational spectrum [17], where$ \hat{Q}_{0} $ is the quadrupole operator in the$ O(6) $ limit. This interesting result was further studied by [18, 19].Inspired by the relationship between γ-rigid triaxial deformation and higher-order interactions, Fortunato et al. investigated triaxiality with a cubic-Q interacting boson model Hamiltonian [20]
$ \hat{H}_{2}=c\left[(1-\eta) \hat{n}_{d}-\eta\left(\frac{\hat{Q}_{\chi}\cdot \hat{Q}_{\chi}}{N}+k\frac{[\hat{Q}_{\chi}\times \hat{Q}_{\chi}\times \hat{Q}_{\chi}]^{(0)}}{N^{2}}\right)\right], $
(2) where k is the coefficient of the cubic term. They state in their paper, "this looks like the simplest one and it is easy to justify on physical grounds as the first higher-order interaction term in an expansion based on the quadrupole operator". This Hamiltonian is only discussed in the large N limit within the intrinsic state formalism and the phase diagram is explored. One key result is that, when
$ \chi=-{\sqrt{7}}/{2} $ in the$S U(3)$ limit, the cubic term corresponds to an oblate shape. Thus, a new evolutional path exists from the prolate shape to the oblate shape (Fig. 1). Based on the results, an analytically solvable prolate-oblate shape phase transitional description within the$S U(3)$ limit was investigated in [21], which offers a finite-N first-order shape transition. Most importantly, the phase transitional point is also a degenerate point [21] (Fig. 2), which may imply a hidden symmetry [22].Figure 2. Evolutional behaviors of the
$S U(3)$ irreps (14,0), (10,4), (6,6), (2,8) for$ N=7 $ in$ \hat{H}^{(3)} $ . The key observation is that the critical point is also a degenerate point.Another key result is that this extended Hamiltonian
$ \hat{H}_{2} $ has only a very small region of rigid triaxiality in the large-N limit at$ \chi\approx -{\sqrt{7}}/{2} $ when the parameter changes from the$ U(5) $ limit to the$S U(3)$ degenerate point (green line in Fig. 1). Thus the shape transitional behaviors from the$ U(5) $ limit to the$S U(3)$ degenerate point will differ significantly from the ones from the$ U(5) $ limit to the$ O(6) $ γ-soft rotation (red line in Fig. 1). Based on these important new findings in Refs. [20, 21], it is very interesting to investigate the spectra of this transitional region for finite-N, which is related to rigid or soft γ-triaxiality.Some experimental requirements remain to deepen our understanding on γ-soft triaxiality and its relationship with the higher-order interactions. In recent experimental investigations, a cluster of extremely neutron-deficient nuclei 168Os [23], 166W [24], 172Pt [25], and 170Os [26] were observed to have an unpredictably small ratio of reduced transition probabilities
$ B_{4/2}=B(E2;4^{+}_{1}\rightarrow 2^{+}_{1})/ B(E2;2^{+}_{1}\rightarrow 0^{+}_{1}) $ along the yrast band. The$ B(E2) $ anomaly is considered a puzzle in the field of nuclear structures and cannot be explained by many existing theories. Recently, the author successfully described the$ B(E2) $ anomaly of the yrast band in 170Os [27] for the first time via adding two third-order$S U(3)$ conserving interactions into the common Hamiltonian used in IBM-1. In this paper, the spectra of the nucleus is γ-soft. This unexpected discovery makes the$S U(3)$ higher-order interactions more important in the interacting boson models.Wilets and Jean first provided a γ-soft solution based on the Bohr geometrical model [28]. When the IBM is determined, its
$ O(6) $ limit can be used to fully describe γ-soft features [29, 30], which is considered a landmark for success of the IBM. However, realistic γ-soft nuclei still cannot be completely described using these models. For example, 196Pt is the first candidate for the$ O(6) $ limit (see the spectra of 196Pt in Fig. 3), but its quadrupole moment is not zero [31].Figure 3. Partial low-lying energy spectra of 196Pt, 110Cd normal states and 120Cd normal states. 196Pt is a typical example of a γ-soft nucleus described by the
$ O(6) $ limit, and there is no a$ 0^{+} $ state near energy levels$ 4^{+}_{1} $ and$ 2^{+}_{2} $ . 110Cd has a typical spherical vibrational spectra, but 120Cd has no the$ 0^{+}_{3} $ state in the three-phonon level.Furthermore, the phonon modes as a major paradigm for description of nuclei near the closed shell have been questioned [32–35] and should be replaced by γ-soft rotation [36]. Figure 3 shows the spectra of the 110Cd normal states, which resembles the spherical spectra in the
$ U(5) $ limit and is different from the$ O(6) $ γ-soft rotation (see the level positions of the$ 0^{+}_{2} $ and$ 0^{+}_{3} $ in 196Pt and 110Cd normal states). In 120Cd (Fig. 3), it is shown that, the$ U(5) $ -like spectra is actually an illusion, and there is no$ 0^{+}_{3} $ state in the three-phonon level [37]. In recent studies [38, 39] the$ 0^{+}_{3} $ state is explained as intruder excitation for the$ 0^{+}_{3} $ state as a band-head of a rotational band has been established in 112Cd. Thus, in the normal states of the Cd isotopes, a$ 0^{+} $ state near the energy level of$ 6^{+}_{1} $ state does not exist. The problem is that the special γ-soft spectra of the normal states cannot be reproduced in the previous IBM Hamiltonian.Recent detailed experimental investigations have revealed that the γ-soft behaviors in 126-132Xe [40–42] and 98-102Zr [43, 44] cannot also be explained using traditional γ-soft descriptions.
These results imply that our understanding of the γ-softness in nuclear structure theories is still incomplete. Searching for a new γ-soft rotational description is vital for our understanding of γ-softness and many theoretical deviations from experimental data. The aspects discussed above make a numerical study of the interacting bosom model with higher-order interactions meaningful: (1) The addition of higher-order interactions may induce new unpredicted phenomena, such as the
$ B(E2) $ anomaly. (2) Rigid triaxiality may be described by this model or its extensions, which is different from the traditional approach discussed in [6, 7] and is important for us to understand γ-rigid triaxial nuclei 76,78Ge [45–47]. (3) Some new insights on γ-soft rotation are required to explain various γ-softness anomalies.In this paper, new γ-soft rotational behaviors are sought. A similar Hamiltonian with the formalism
$ \hat{H}_{2} $ is investigated numerically.$ U(5) $ -like and$ O(6) $ -like γ-soft spectra are discovered, which can have large quadrupole moments. An unexpected partial$ O(5) $ dynamical symmetry is observed. The$ U(5) $ -like spectra is applied in 110Cd normal states, which can reproduce the type of the normal states. -
Our aim is to search for new γ-soft rotation, which is compared with the traditional γ-soft behaviors in the transitional regions from the
$ U(5) $ limit to the$ O(6) $ limit; therefore, the parameters are selected as in the triangle in Fig. 1. A direct numerical calculation of the cubic-$ \hat{Q}_{\chi} $ interacting boson model Hamiltonian$ \hat{H}_{2} $ [20] is possible, but their spectra appear to lack regularity. To determine the hidden structure associated with the$S U(3)$ degenerate point, a new formalism should be developed. This new Hamiltonian consists of three parts. The first part is the common d boson number operator$ H^{(1)}=\hat{n}_{d}=d^{\dagger}\cdot \tilde{d} $ in the$ U(5) $ limit, which produces the simple harmonic vibration. The second part is the quadrupole-quadrupole interaction$ H^{(2)}=-\hat{Q}_{0}\cdot \hat{Q}_{0}/N $ in the$ O(6) $ limit, which produces the typical solvable γ-soft spectra. The combination of the two parts can describe the shape transitions from spherical to traditional γ-soft nuclei. The critical point of this transitional region can be described using$ E(5) $ dynamical symmetry [48]. A typical feature of γ-softness is the level degeneracy between the ground-band and quasi-γ rotational band due to the common$ O(5) $ symmetry, such as$ 4^{+}_{1},\;2^{+}_{2} $ or$ 6^{+}_{1},\;4^{+}_{2},\;3^{+}_{1} $ (Fig. 3).When the third part is included, such as the quadrupole-quadrupole interaction
$ -\hat{Q}\cdot \hat{Q}/N $ in the$S U(3)$ limit, γ-softness is destroyed, and the level degeneracy between the ground-band and quasi-γ band is removed [1]. It appears the framework of the IBM-1 offers no opportunity for a new γ-soft description. Since the emergence of the interacting boson model nearly fifty years ago, the γ-softness is always related to the$ O(6) $ dynamical symmetry.The numerical results in this paper reveal that it is not the case. Here, the third part is a combination of the
$S U(3)$ second-order and third-order Casimir operators,$ \hat{H}^{(3)}= -\frac{\hat{C}_{2}[S U(3)]}{2N}+\kappa \frac{\hat{C}_{3}[S U(3)]}{2N^{2}}, $
(3) which is investigated in detail in Ref. [21]. The two Casimir operators have relationships with the quadrupole second or third-order interactions in the
$S U(3)$ limit as follows:$ \hat{C}_{2}[S U(3)]=2\hat{Q}\cdot \hat{Q}+\frac{3}{4} \hat{L}\cdot \hat{L}, $
(4) $\begin{aligned}[b] \hat{C}_{3}[S U(3)]=&-\frac{4}{9}\sqrt{35}[\hat{Q}\times \hat{Q} \times \hat{Q}]^{(0)}\\&-\frac{\sqrt{15}}{2}[\hat{L}\times \hat{Q} \times \hat{L}]^{(0)}.\end{aligned} $
(5) For a given
$S U(3)$ irrep$ (\lambda,\mu) $ , the eigenvalues of the two Casimir operators under the group chain$U(6)\supset S U(3) \supset O(3)$ are expressed as$ \langle \hat{C}_{2}[S U(3)]\rangle=\lambda^{2}+\mu^{2}+\lambda \mu+3\lambda+3\mu, $
(6) $ \langle \hat{C}_{3}[S U(3)]\rangle=\frac{1}{9}(\lambda-\mu)(2\lambda+\mu+3 ) (\lambda+2\mu+3 ). $
(7) Thus, in the
$S U(3)$ limit,$ \hat{H}^{(3)} $ is solvable, which has a critical point at$ \kappa_{0}={(3N)}/{(2N+3)} $ , (Fig. 2, when N=7,$ \kappa_{0}\approx 1.24 $ ). Note that each irrep$ (\lambda,\mu) $ corresponds to a special quadrupole deformation [9, 10]. When$ \kappa < \kappa_{0} $ , it presents a prolate shape, and when$ \kappa >\kappa_{0} $ , it is (nearly) an oblate shape. This shape phase transition is abrupt at the critical point. Importantly, the critical point is also a multiple-phase coexistence or degenerate point (Fig. 2). At this degenerate point, the$S U(3)$ irreps satisfying the condition$ \lambda+2\mu=2N $ are all degenerate, and the degeneracy degree is${(N+2)}/{2} $ for an even N or$ {(N+1)}/{2} $ for an odd N. This degeneracy observed here is not accidental; thus, it may imply a hidden symmetry [22]. This degenerate point may be related to the important studies of Sebe and Akiyma, which are briefly discussed in Section VI. The Hamiltonian with$ \kappa_{0}={(3N)}/{(2N+3)} $ is adopted to the third part and is denoted as$ \hat{H}^{(3)} $ .Now, we discuss the full Hamiltonian for the new γ-soft deformation, which is expressed as
$ \begin{eqnarray} \hat{H}=c[(1-\eta) H^{(1)}+\eta((1-\xi) H^{(2)}+\xi H^{(3)})], \end{eqnarray} $
(8) where
$ 0\leq \eta \leq 1 $ , and$ 0\leq \xi \leq 1 $ . When$ \eta=0 $ , it is the$ U(5) $ limit. When$ \eta=1, \xi=1 $ , it represents the degenerate point in the$S U(3)$ limit, and when$ \eta=1, \xi=0 $ , it is the$ O(6) $ limit (Fig. 1). The Hamiltonian is numerically investigated using the diagonalization method based on the$S U(3)$ interaction [3, 27]. -
The
$ B(E2) $ values are necessary for us to understand the γ-softness. The operator is defined as$ \hat{T}(E2)=e\hat{Q}_{\chi}, $
(9) where e is the boson effective charge and
$ \chi=-{\sqrt{7}}/{2}\xi $ . The evolutional behaviors of the$ B(E2; 2_{1}^{+}\rightarrow 0_{1}^{+}) $ ,$B(E2; 0_{2}^{+}\rightarrow 2_{1}^{+})$ ,$ B(E2; 0_{2}^{+}\rightarrow 2_{2}^{+}) $ ,$ B(E2; 0_{3}^{+}\rightarrow 2_{1}^{+}) $ , and$ B(E2; 0_{3}^{+}\rightarrow 2_{2}^{+}) $ values are plotted in Fig. 7 when η changes from 0.0 to 1.0 and$ \xi=0.0 $ (a),$ \xi=0.5 $ (b), and$ \xi=1.0 $ (c). The transitional behavior of the$ B(E2; 2_{1}^{+}\rightarrow 0_{1}^{+}) $ value is similar to the one from the$ U(5) $ limit to$ O(6) $ limit. The values of the$ B(E2; 0_{2}^{+}\rightarrow 2_{1}^{+}) $ are reduced whereas the ones of the$ B(E2; 0_{2}^{+}\rightarrow 2_{2}^{+}) $ are promoted. The values of the$ B(E2; 0_{3}^{+}\rightarrow 2_{2}^{+}) $ are also reduced. These are all the typical trends for the γ-soft rotation (Fig. 8).Figure 7. (color online) Evolutional behaviors of
$ B(E2; 2_{1}^{+}\rightarrow 0_{1}^{+}) $ (green solid line),$ B(E2; 0_{2}^{+}\rightarrow 2_{1}^{+}) $ (blue solid line),$ B(E2; 0_{2}^{+}\rightarrow 2_{2}^{+}) $ (blue dashed line),$ B(E2; 0_{3}^{+}\rightarrow 2_{1}^{+}) $ (red solid line), and$ B(E2; 0_{3}^{+}\rightarrow 2_{2}^{+}) $ (red dashed line) when η changes from 0.0 to 1.0 and (a)$ \xi=0.0 $ , (b)$ \xi=0.5 $ , and (c)$ \xi=1.0 $ for$ N=7 $ .Figure 8. (color online) Evolutional behaviors of
$ B(E2; 2_{1}^{+}\rightarrow $ $ 0_{1}^{+}) $ (green solid line),$ B(E2; 0_{2}^{+}\rightarrow 2_{1}^{+}) $ (blue solid line),$B(E2; 0_{2}^{+}\rightarrow $ $ 2_{2}^{+})$ (blue dashed line),$ B(E2; 0_{3}^{+}\rightarrow 2_{1}^{+}) $ (red solid line), and$ B(E2; 0_{3}^{+}\rightarrow 2_{2}^{+}) $ (red dashed line) when ξ changes from 0.0 to 1.0 and$ \eta=1.0 $ for$ N=7 $ .Now, we discuss the transitional pattern for the quadrupole moment of the
$ 2^{+}_{1} $ state, which is shown in Fig. 9. This quantity in the$ O(6) $ limit is absolutely zero. If a$S U(3)$ two-body interaction is mixed, a large value can be obtained, but the γ-soft degeneracy will be significantly destroyed. This confusion has existed for many years. Specifically, this quantity is related to the first excited state, which is vital for a successful model [31]. Fig. 9 shows that the values increase when ξ changes from 0 to 1 for$ \eta=1.0 $ , which may resolve the debates between γ-softness and large quadrupole moment. -
The
$ U(5) $ -like softness can be used to fit the spectra of 110Cd normal states, and the$ \hat{L}^{2} $ term is also incorporated. The Hamiltonian is$ \hat{H}'=\alpha H^{(1)}+\beta H^{(3)}+\gamma \hat{L}^{2}, $
(10) here
$ \xi=1.0 $ ,$ \alpha=c(1-\eta) $ ,$ \beta=c\eta $ , and γ is the coefficient of the$ \hat{L}^{2} $ term. Fig. 10 shows the partial low-lying levels for 110Cd normal states. The fitting results reproduce the style of experimental data; however, for higher-levels, the theoretical values are larger than the experimental ones. To reduce the energies of the higher-levels, Pan et al. presented a new method and observed an excellent fitting result for 194Pt [49], which may be considered in future research to improve the fitting precision. The theoretical energy of the$ 0^{+}_{3} $ state is 3411.21 keV, which is significantly larger than the energy of the$ 6^{+}_{1} $ state, smaller than the$ 6^{+}_{2} $ state, and nearly twice the energy of the$ 0^{+}_{2} $ state. Experimentally, a$ 0^{+} $ state exists with an energy of 2662 keV, which is between the energies of the$ 6^{+}_{1} $ state (2480 keV) and$ 6^{+}_{2} $ state (2877 keV).Figure 10. Partial low-lying levels for 110Cd normal states. The values above are the experimental data and the ones below are the results of theoretical fitting.
The
$ B(E2) $ values of the lowest levels are compared with the experimental results of the normal states in 110Cd, which are listed in Table 1. This γ-soft description can produce a good consistency with the empirical data qualitatively, which is different from the phonon descriptions. The quadrupole moment of the$ 2^{+}_{1} $ state is$ - $ 0.36 eb, which is also close to the experimental value of$ -0.39 $ eb. When weak mixing with the intruder states is considered, more reasonable results may be obtained [36]. Thus, our Hamiltonian may be also vital for understanding the Cd puzzle [51].$ L_{i} $ $L_{f} $ Expt. Results $ 2_1^+ $ $0_1^+ $ 27.0(8) 27.0 $ 4_1^+ $ $2_1^+ $ 42(9) 39.0 $ 2_2^+ $ $2_1^+ $ $30(5);\;19(4) ^{\rm a}$ 39.8 $0_1^+ $ $1.35(20);\;0.68(14) ^{\rm a}$ 0.17 $ 0_2^+$ $2_1^+ $ $<7.9 ^{\rm a} $ 12.2 $2_2^+ $ < 1680a 59.5 $ 6_1^+$ $4_1^+ $ $40(30);\;62(18) ^{\rm a}$ 44.3 $4_2^+ $ $<5 ^{\rm a} $ 3.08 $ 4_2^+$ $4_1^+ $ $12 ^{+4}_{-6};\;{10.7^{+4.9}_{-4.8}}^{\rm a}$ 21.1 $2_1^+ $ $0.20 ^{+0.06}_{-0.09} ;\;0.14(6) ^{\rm a}$ 0.04 $2_2^+ $ $32 ^{+10}_{-14} ;\;22(10) ^{\rm a}$ 23.2 $ 3_1^+$ $4_1^+ $ $5.9^{+1.8}_{-4.6} ;\; {2.4^{+0.9}_{-0.8}}^{\rm a}$ 12.9 $2_1^+ $ $1.1^{+0.3}_{-0.8} ;\;0.85(25) ^{\rm a}$ 0.11 $2_2^+ $ $32^{+8}_{-24} ;\;22.7(69) ^{\rm a}$ 31.5 $ 2_3^+$ $4_1^+ $ $ <5 ^{\rm a} $ 5.95 $2_1^+ $ $ 2.8^{+0.6}_{-1.0} $ 0.08 $2_2^+ $ ${{0.7} ^{+0.5}_{-0.6}}^{\rm a}$ 3.62 $0_2^+ $ 24.2(22)a 24.2 a From Ref. [36].
New γ-soft rotation in the interacting boson model with SU(3) higher-order interactions
- Received Date: 2022-01-24
- Available Online: 2022-07-15
Abstract: The interacting boson model with